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Professor Spurgeon's papers comprise mainly notes, 1895-1912, taken at lectures attended as an undergraduate and afterwards, and teaching notes and course syllabuses, 1901-1927, relating to lectures given at Bedford College and elsewhere, including for London County Council evening classes. She kept two volumes of notes on the students she taught at Bedford College, and one letter survives (PP7/1/3/8) expressing appreciation for her teaching. There are papers relating to her research in English literature, including on Chaucer, mysticism, Ruskin, Shakespeare and Keats, [c.1900]-1933, and published copies of her works, 1901-1930, some with annotations. She collected newspaper cuttings on literature and her own work, and on current affairs, including feminism and women's suffrage and the First World War. There are papers relating to her work on international exchange of information about education, particularly for women, including her presidency of the International Federation of University Women, 1920-1924, and the British Federation's establishment of Crosby Hall International Hall of Residence, 1921-1929. There is one file of letters, cards and notes found in her books, 1889-1936, including letters from and to Frederick James Furnivall, founder of the Early English Text Society, Chaucer Society, Ballad Society, New Shakespeare Society, etc, and letters and cards from Edmund Gosse, Emile Legouis, Professor of English Literature at the Sorbonne, and George Heynes Radford (later Sir George Radford, Labour M.P. for East Islington). Two files of letters from CS to her aunt Mrs E. Harvey 1898-9, 1905-1914, were added to the papers in 1964. There is also a typed copy of Professor Spurgeon's will and bequest to Bedford College, 1936.