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The majority of the collection is made up of journals kept by Buckle during the years 1866-1870, during which he travelled to South America, South Africa and Australia (there are also periods during which he was stationed at Portsmouth). There are some lacunae in the sequence of diaries. There is also one autograph album kept by Buckle relating partly to his own affairs (his application to become House Surgeon at the West Norfolk and Lynn Hospital, 1863-1864) but also including older material predating his birth.