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The collection includes Schiller's notebooks, his working notes, scripts of his lectures, articles and essays, correspondence concerning engagements and with colleagues and students, material relating to his involvement with courses for teachers, personalia, printed material and photographs. Schiller's notebooks mainly contain working notes and the text for his lectures which provide evidence of his educational ideas, for instance, on the teaching of numbers, the importance of freedom and creativity through art, craft and movement activities, on reading, writing and conversation.
Also included are the notes and papers of Schiller's wife, Mrs Lyndall Schiller, including diaries of their daughters' childhood development. These records of Lyndall were deposited along with those of her husband and as much of them relate to matters that were of interest to both of them they have been retained within the collection of her husband's papers.
In addition the collection contains papers of two of Schiller's students who attended the 'Course on the Education of Children in the Junior School' organised by Christian Schiller at the University of London Institute of Education, 1959s. These include some wooden mathematical teaching apparatus.

This collection comprises slides used by Ivor Pfuell in his lectures on the history and development of London. The slides were collected during the 1970s and 1980s, although they depict London locations and landmarks through the ages.

Papers of Ian Michael, including material relating to his time at the University of Malawi and subsequent visits, including correspondence, policy papers, pamphlets, programmes, maps and other printed material, 1964-1990; published and unpublished papers relating to African education, 1966-1981.
Material relating to his research on the history of the teaching of English, including files of notes comprising transcripts from, summaries of, and comments on, a range of works connected with the teaching of English; card indexes forming a working bibliography of books mainly related to the teaching of English up to 1870, but also including some Latin texts, other curriculum subjects and more modern texts.

Letter from Baldassarre Boncompagni-Ludovisi, 1858, [To Augustus De Morgan]. Thanking De Morgan for his letter of 14 November 1858, giving information about Francesco Galigai's 'Pratica d'Arithmetica' (1548), and asking for further details. Letter enquires about the library of Dr [Daniel Mitford] Peacock and asks De Morgan to get Count [Guglielmo] Libri to send catalogues of sales he was to hold [in March and August 1859] in England and in Paris. Enquires about further editions of De Morgan's 'Arithmetical Books' (1847) and offers to get one printed in Rome.

Extensive collection of personal and working papers reflecting many aspects of Joseph Lauwerys' varied career, including science education, educational broadcasting, international co-operation and understanding and comparative education. They include correspondence files, mostly dating from the late 1940s onwards; lecture notes, articles, conference papers and other published and unpublished writings; files relating to societies, associations and organisations; material about post-War reconstruction and the founding of UNESCO; files relating to specific overseas visits and tours; and collected papers on the educational conditions in many different countries.

Papers of Rose Kosky, [1970s-1980s], chiefly relating to the Barking Reading Project, including schemes, cassettes, notes and teaching materials.

Records of Annie Horatia Jones, daughter of Sir Horace Jones. The collection contains ten dolls' house dolls dressed by Tamazine Billings (nee Jones) in 1886 for her niece, Annie Horatia Jones, to represent members of Sir Horace Jones' family and household. The dolls' original labels have been sewn onto their clothing to identify the family member they are intended to represent. There is also a photograph album depicting family including Sir Horace Jones, portrait of Annie Horatia Jones in outfit for City of London Mansion House Juvenile Dress Ball, and family at home in Devonshire Place; her correspondence with aunts, housekeeper and friends concerning holidays, her pursuits and interests (1883-1890), a scrapbook of coloured pictures and also a pencil drawing of Tamazine Billings as a girl (circa 1831). The collection presents an insight into Sir Horace Jones' family life. The different heights of the dolls of Sir Horace Jones and Lady Ann Elizabeth Jones and the size of dolls is thought to represent other family members demonstrates Victorian attitudes towards personal status within the family. The clothing on the dolls is also useful for looking at costume and dress during the late nineteenth century.

Adult Education VHS videos: "Teaching English as a second language in the Post School Sector", 1985 and "Teaching adult literacy Unit A: A mixed ability class", 1980s.

Papers of John Henley comprising notes of lectures delivered in London on historical, political and religious subjects.

This collection mainly consists of personalia including educational certificates, school reports, examination papers, and notebooks of William Joseph George Hands' mathematical studies at Cambridge. It includes a small amount of ephemera relating to the Board of Education Exhibition which took place in connection with the Imperial Education Conference, 1923 and to the activities of the International Educational Society. Also included are a paper by Hands on 'A simplified curriculum based on occupations', 1925, and papers on experiments with English composition at St Mary's Boys' School, Weymouth and with the topical treatment of history and geography at S. Aldhelm's Girls' School, Branksome, c.1910.

Personal papers of Canon Samuel Augustus Barnett, social reformer. The papers comprise correspondence, sermons and lecture notes, and miscellanea. The bulk of the correspondence consists of weekly letters from the Canon to his brother, Francis G. Barnett and, after the latter's death, to his widow and her daughter and sons. For the years before 1883 there are no letters at all, and before 1889 there are fewer than for the later years of the correspondence. Normally the Canon wrote every Saturday, but there are frequent periods when there was no correspondence, when the Canon was in residence at Bristol during the summers of 1893-1906, and when the two families were holidaying together. There are also large groups of letters written by the Canon to his mother and family in the form of travel journals during his trips to Egypt in 1879-1880 and round the world in 1890-1891.

There are very few in-letters. The letters to F G Barnett are almost always four octavo pages in length. They were bundled in one or two year periods by Dame Henrietta when preparing her biography of her husband. On several letters there are editorial instructions, deletions and emendations by Dame Henrietta. These were made in pencil and were, at some subsequent period, erased. Within each bundle Dame Henrietta also numbered the letters. Her numbering has not been indicated in the list, nor has it been followed, as several of the letters were in fact misplaced.

There is a series of bound sermon notebooks and miscellaneous lecture notes amongst these papers. Although the sermon notes are basically complete for the St. Jude's period, 1875-1888, the lecture notes are only a fraction of the Canon's output.

Some miscellaneous documents and in-letters were kept by the Canon for their intrinsic importance, e.g. formal documents relating to his benefice at St. Jude's, and these have survived. There are, in addition, miscellaneous photographs, mostly of the Canon, but also of his wife and of his family.

These papers will be of interest to historians for the information they give on Canon Barnett's life, and for the frequent and lengthy discussions of the political, social and intellectual life of the day. They are enhanced in value by the fact that Dame Henrietta was avowedly unable to do them more than scant justice in her life of the Canon (see Canon Barnett: his life, work and friends vol I, p.377), and that the records of Toynbee Hall have been decimated by war damage and destruction.

Papers collated by Gene Adams relating to her work in museums education, especially for the Inner London Education Authority (ILEA) including:
Publications written by Adams relating to museums education [1970s]-1990; papers relating to her work as an art teacher, including writings by pupils and photographs of their work,1960s; papers relating to her educational work at the Geffrye Museum, [1959]-1975; papers relating to her work on various projects relating to the Spitalfields area, 1976-1996, including the Spitalfield trail and related activities created for the Geffrye Museum, conservation of the Spitalfields area, and an exhibition on the history of the area to raise awareness of its endangered architecture which later became a travelling exhibition; papers regarding her work on museums education for ILEA, [1975]-1990, including correspondence, education project based at the historic houses of the Greater London Council (GLC), projects Adams' worked on for other museums in London, in-service teacher training course in museums, the 'Museum Visits' guide including the museum charts, a museums index, survey of the usage of London museums by schools, other surveys relating to museums, correspondence regarding her advisory service for London museums, and other files; papers regarding her work as a freelance educational advisor, 1988-1999; sound and visual recordings relating to her work for the Geffrye Museum and ILEA, [1972-1988]; collection of photographic slides of her educational work mostly relating to her work for the Geffrye Museum, ILEA and images relating to the Spitalfields exhibition, [1974-2002]; general publications collected by Adams during her research on education on museums, including leaflets and teachers packs created by local area museum services or individual museums in the UK and abroad and press cuttings.