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Papers of Sir Sydney Caine, [1955-1968], notably material on the early history of the London School of Economics, [1955-1958], including copies of articles by Lady Janet Beveridge concerning the administration of the LSE following World War One and the Directorship of William Henry Beveridge, 1st Baron Beveridge of Tuggal; papers relating to Caine's Directorship of the LSE, 1966-1969, mainly comprising material relating to student unrest; two volumes of a personal diary, 1942-1943; a photograph album of the West Indian Sugar Commission, 1929-1930.

Papers and notes by Professor Lakatos on the philosophy of mathematics and science, including notes on Feyerabend, Kuhn and Popper; correspondence with many academics and philosophers; papers relating to the International Colloquium on the Philosophy of Science organised by Lakatos in 1965; and biographical material, desk diaries, press cuttings, and papers relating to student politics and the LSE 'troubles'.

Papers of Sir Gilbert James Morley Longden. Comprised of general political correspondence and papers; constituency papers; subject files; political writings; collected published material; personal memorabilia, correspondence and papers; autobiographical material; papers about the collection; 1901-1996.

Papers of Lionel Charles Robbins, Baron Robbins of Clare Market, 1930-1937 and 1968-1970, comprising material concerning his membership of the Committee of Economics (a sub-group of the Economic Advisory Committee), 1930-1937, including minutes and agenda, correspondence with John Maynard Keynes and Hubert Douglas Henderson, and duplicated papers and reports by Keynes, Arthur Cecil Pigou and Henderson; papers relating to the LSE 'Troubles', 1968-1970, including copies of documents released in connection with student disturbances and notes of the proceedings of the LSE Appeals Committee.