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Papers of Lyon Playfair, 1st Baron Playfair of St Andrews, 1795-1910, comprising general correspondence, 1795, 1840-1910, covering a range of subjects relating to Playfair's scientific and political interests, notably with Prince Albert, 1851-[1853], and via Charles Grey, 1850-1861, concerning the Great Exhibition, Alfred, Duke of Edinburgh, 1865-1886, Matthew Arnold, 1883, Sir Charles Barry, 1795-1860, Thomas Francis Bayard, concerning 'Venezuela dispute', 1896, Queen Victoria, 1883, and via Sir Arthur John Bigge, 1895-1898, Charles Booth, 1895, Sir David Brewster, concerning lighthouses,1851-1868, Robert Wilhelm Bunsen, concerning their research, 1841-1849, Edwin Chadwick, concerning agriculture and politics, 1855-1899, concerning pensions, Joseph Chamberlain, concerning the Aged Poor Commission, Venezuela, 1894-1899, Prince Christian of Schleswig-Holstein, concerning the 1851 Commission,1882-1896, Sir Robert Christison, concerning vivisection bill, 1867-1876, Anthony Ashley Cooper, 1852-1874, Charles Darwin, concerning vivisection bill, 1875, Sir Thomas Henry De La Beche, concerning the Geological Survey, 1842-1852, Sir James Dewar, 1885-1898, Albert Edward, Prince of Wales (later Edward VII), 1879-1898, Michael Faraday, 1842-1857, William Ewart Gladstone, 1859-1892, Thomas Graham, 1839-1867, Thomas Henry Huxley, 1854-1891, Henry James, 1898, George Granville Leveson-Gower, [1850]-1889, Justus von Liebig, 1841-1873, Joseph Lister, 1876-1898, David Livingstone, including an account of his exploration in Africa, 1861, John Stuart Mill, 1868, Viscount Horatio Nelson to 'Pollard', 1795, Sir Robert Peel, [1842]-1850, letters of condolence to Lady Playfair on the death of Lord Playfair, 1898.

Family correspondence, comprising letters to various correspondents from Playfair, 1854-1898, notably his son George and daughter-in-law; letters from Edith Playfair (third wife), to her step-son, 1898.

Papers relating to diplomas and appointments, 1840-1892, notably appointment as Professor of Chemistry, Edinburgh University, 1858, Charity Commissioner, 1886, Lord-in-Waiting to Queen Victoria, 1892, Privy Councillor, 1873.

Papers relating to orders and decorations, 1851-1898, notably Order of the Bath, Order of the Legion of Honour and Jubilee Medal.

Papers of Lord Willis Jackson, 1916-1970, comprising papers transferred from his office in Imperial College, namely personal and biographical papers, 1923- 1970, including student notebooks, [1923], visits abroad, 1961-1968, speeches and addresses, 1950-1970, family correspondence, Parliamentary correspondence, 1957-1970, photographs [1916]-1967, mainly of official events, laboratories and apparatus, Willis Jackson; papers relating to Associated Electrical Industries and Metropolitan-Vickers, 1951-1969, notably appointment as Director of Research and Education, 1953, correspondence and press cuttings, 1951-1969, engineering and staff courses, 1954-1959; papers relating to Imperial College, 1950-1969, notably lectures and speeches, 1950-1968, correspondence, 1953-1970, including with Professor Colin Cherry, 1950-1969, the Rector, Lord Penney, 1967-1970, papers concerning academic matters, 1955-1968, Committees, 1963-1969, societies and associations, 1950-1970, Electrical Engineering Department, 1964-1969; correspondence with Ministers, reports and papers relating to Government Departments, principally concerning committees and advisory councils, 1944-1970, notably the Admiralty (later Ministry of Defence), 1950-1968, Ministry of Education, 1954-1969, Ministry of Technology, 1965-1970, Department of Scientific and Industrial Research, 1944-1965, Ministry of Overseas Development, 1965-1969, Organisation for Economic Cooperation and Development (ORCD), 1961-1969, University Grants Committee, 1953-1969, Royal Commission on the Civil Service, 1953-1958, Delhi Institute of Technology, 1957-1970; correspondence, reports and committee papers relating to the Institution of Electrical Engineers, 1950-1968; correspondence, 1950-1970, notably with professional institutions and associations, such as the Association of Supervising Engineers, 1960-1968, Educational establishments, notably the University of London, 1953-1970, Manchester Institute of Science and Technology, 1951-1970, Sir Eric Ashby, 1959-1966, Bertram Vivian Bowden, 1958-1968, Patrick Maynard Stuart Blackett, 1957-1969, British Broadcasting Corporation (BBC), 1961-1969, Sir John Douglas Cockcroft, 1953-1964, Dennis Gabor, 1951-1969, Sir Harold Hartley, 1961-1968, Eric Balliol Moullin, 1953-1958, Kathleen Mary Ollerenshaw, 1958-1964, John Arthur Saxton, 1960-1967, Joseph Sidney Weiner, 1967-1968.

autobiographical scrapbooks, 1916-1970, from Lady Jackson, comprising 91 loose-leaf binders compiled from 1952, containing heterogeneous papers, including photographs, biographical material such as letters of appointment, comments and narratives, manuscript and published texts of lectures and speeches, press cuttings, social correspondence, travel schedules and reports on visits.