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The collection mainly consists of a set of Isabel Fry's personal diaries and notebooks dating from 1878-1958. These are supplemented by letters to her friend Eugénie Dubois, c1930-1958, and a few publications and photographs. The diaries reflect all aspects of her life and career including her teaching activities and educational ideas; her preoccupations with political and social affairs, including political reform and emancipation in the East and in Turkey and Persia; her friendships with liberal intellectuals; and her involvement with anti-militarist movements, slum clearance, socialism and feminism. Also included are details of her relationship with her family, friends and their wider social circle.

Papers of Harold and Pamela Silver, mainly research material for An Educational War on Poverty including: audio-cassettes of 41 taped interviews and some manuscript interview notes, 1981-1982; published and unpublished reports, articles and research papers relating to educational programmes and initiatives in the United States and Britain, 1950s-1980s; correspondence and papers (mainly photocopies) of A.H. Halsey and Michael Young relating to the National Educational Priority Area Projects, 1967-1972; articles, reports and correspondence relating to the report of the Central Advisory Council for Education (England) Committee of Enquiry into Primary Education, Children and Their Primary Schools (The Plowden Report), including some papers of Maurice Kogan, 1963-1987.

Records of the Society of Teachers Opposed to Physical Punishment, [1968-1989], including press cuttings, letters to the press, press releases, publications, case files, administrative, policy and subject files.

Papers of The Moot, mainly consisting of Sir Fred Clarke's set of the circulated discussion papers, 1939-1942; also an incomplete run of the Christian News-Letter, 1939-1949.