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The collection includes Schiller's notebooks, his working notes, scripts of his lectures, articles and essays, correspondence concerning engagements and with colleagues and students, material relating to his involvement with courses for teachers, personalia, printed material and photographs. Schiller's notebooks mainly contain working notes and the text for his lectures which provide evidence of his educational ideas, for instance, on the teaching of numbers, the importance of freedom and creativity through art, craft and movement activities, on reading, writing and conversation.
Also included are the notes and papers of Schiller's wife, Mrs Lyndall Schiller, including diaries of their daughters' childhood development. These records of Lyndall were deposited along with those of her husband and as much of them relate to matters that were of interest to both of them they have been retained within the collection of her husband's papers.
In addition the collection contains papers of two of Schiller's students who attended the 'Course on the Education of Children in the Junior School' organised by Christian Schiller at the University of London Institute of Education, 1959s. These include some wooden mathematical teaching apparatus.

Papers of the Board of Education Inspectors' Association (later the Association of Her Majesty's Inspectors of Schools), 1871-1992, including annual reports, minutes and papers of the Executive Committee and Divisional Committees, reports and memoranda, 1920-1992; lists of Divisions, Districts and staff, issued by the Education Department, 1871-1946; collected personal papers of individual HMIs; material gathered for a post-war history of the Inspectorate.

Records of the Institute of Education, University of London, 1890s-1994 (Ref: IE), including the London Day Training College Local Committee and Council, 1904-1931 (Ref: IE/TCC); Jubilee Lectures correspondence, 1904-1952 (Ref: IE/JUB); the Islington Day Training College, 1906-1917 (Ref: IE/ISL); examination records, 1909-1970s (Ref: IE/EXN); the University of London Training Colleges Delegacy, 1928-1948 (Ref: IE/TCD); the Institute of Education Delegacy, 1931-1948 (Ref: IE/ULD); the Committee of Management, 1948-1987 (Ref: IE/COM); the Council, 1948-1982 (Ref: IE/COU); the Senate, 1987-1992 (Ref: IE/SEN); the Committee of Principals, 1948-1979 (Ref: IE/CPR); Directorate material, including annual report files, 1933-1980 (Ref: IE/ARP), collegiate files, 1925-1975 (Ref: IE/DCO), files of Sir Percy Nunn, 1923-1936 (Ref: IE/TPN), the papers of G.B. Jeffery, 1940s-1950s (Ref: IE/GBJ), subject files, 1950s-1980s, and letter books, 1906-1926 (Ref: IE/PLB); Secretariat day files, 1948-1984 (Ref: IE/DLB), and subject files, 1960s-1990s, and memoranda books, 1907-1937 (Ref: IE/MEM); the Central Academic Board, 1949-1987; the Meeting of Staff and the Academic Board, 1909-1982 (Ref: IE/CAB, IE/ACB, IE/ABD); the Department for Overseas Students, 1930s-1980s (Ref: IE/DOS); visitation files, 1949-1971 (Ref: IE/VIF), and papers of the Visitations Sub-Committee, 1948-1969 (Ref: IE/VSC); the Conference of Local Education Authorities, 1948-1979 (Ref: IE/LEA); the Domestic Subjects Group of the Training Colleges Delegacy, 1928-1948 (Ref: IE/DSG); research material collated by C. Willis Dixon during the writing of his history of the Institute, 1930s-1970s (Ref: IE/DIX); the Committee on Facilities for Practising Teachers, 1949-1978 (Ref: IE/FPT); the Centre for Teachers, later the INSET Office, 1950s-1990s (Ref: IE/CFT); the Colonial Department, later known as the Department of Education in Tropical Areas, the Department of Education in Developing Countries, and the Department of International and Cooperative Education, 1935-1980s (Ref: IE/COL); the Department of Child Development and Educational Psychology, 1972-1987 (Ref: IE/CDE); the Department of History, Humanities and Philosophy, 1980s-1990s (Ref: IE/HHP); the Department of Mathematics, Statistics and Computing, 1980s-1990s; the Music Department, 1980s; the Library, 1923-1980s, the School Relations Office, 1960s-1980s (Ref: IE/SRO); the Policy Advisory Committee, 1970-1983 (Ref: IE/PAC); the Joint Committee in Education, 1975-1982 (Ref: IE/JCE); the Joint Degree Committees, 1975-1980 (Ref: IE/JDC); the Joint Professional Committee, 1977-1983 (Ref: IE/JPR); the Interim Joint Planning Committee, 1982-1987 (Ref: IE/IJP); the Academic Policy Committee, 1983-1987 (Ref: IE/APC); the Audit Committee, 1991-1993 (Ref: IE/AUD); the Computing Policy Committee, 1988-1992 (Ref: IE/CPC); the Joint Planning Committee, 1988-1994 (Ref: IE/JPC); the Standing Committee on Equal Opportunities, 1987-1993 (Ref: IE/EQO); the Finance and General Purposes Committee, 1988-1992 (Ref: IE/FGP); the Investments Sub-Committee, 1988-1992 (Ref: IE/ISC); the Consortium for Assessment and Testing in Schools, 1980s-1990s; files relating to Institute publications, 1940s-1980s (Ref: IE/PUB); the Institute of Education Society, 1980s; student records, 1902-1980s (Ref: IE/STU); John Adams Hall, 1980s; the Institute Nursery, 1975-1980 (Ref: IE/NUR); research files, 1960s-1980s (Ref: IE/SRF); staff records, 1912-1933 (Ref: IE/SFR); the Senior Common Room, 1960s-1980s (Ref: IE/SCR); photographs (Ref: IE/PHO); Library Committees, 1923-1977 (Ref: IE/LSC); Student Associations/Unions, c1950-c1979 (Ref: IE/SAU); Teacher Training Enquiry [1970-1971] (Ref: IE/TTE); papers of Richard Goodings, c1890s-1960s (Ref: IE/RGO); buildings and estates records (Ref: IE/BLD); charters and statutes (Ref: IE/CSS); History of the Institute Panels (Ref: IE/HIP); records of Peter Newsam (Ref: IE/NEW); records of Peter Mortimore (Ref: IE/PEM); Personnel Department records (Ref: IE/PER); records of a Centre for Higher Education Research project on quality assurance in higher education (Ref: IE/QUR).

Administrative records of the College of Preceptors and College of Teachers, 1847-2008. Including constitutional, legal and membership records, 1847-1998; published calendars and registers, 1880-1940 and 1972-1987; Council records, 1848-1979; committee records including the finance committee, 1874-1966; examinations committee, 1885-1958; Education[al] committee, 1874-1919; Affiliation Committee, 1919-1920; special committees, 1885-1967; Executive Committee, 1931-1946; academic board, 1968-1981; Finance and General Purposes/Educational Times Committee, 1913-1980; House Committee, 1957-1964; Advisory Boards, 1955-1980; and Constitution Committee, 1979; financial records, 1874-1944; examination records, [1860]-1962; press cuttings, 1914-1974; papers regarding conferences and events, 1896-1945; publications, 1847-2010; administrative papers of the College of Teachers, 1997-2002; photographs and illustrations, [1754-1990s]; and papers and photographs relating to award ceremonies, 1973-1992. there is also a small amount of mixed-media material and information relating to historical studies of the College.

The Katherine Bathurst Papers, 1891-1932, focusing mainly on her career at, and disputes with, the Board of Education, her interests in nursery education, the working conditions of the school inspectorate and the position of women within the inspectorate. The papers comprise inspection notes from school visits; notes for her preliminary and supplementary reports; copies of Board of Education Circulars; photocopies of the Women Inspectors' Reports; correspondence with her superiors and officials at the Board of Education; private correspondence, including with Sir John Gorst; correspondence with the National Union of Women Teachers (NUWT) and National Union of Teachers (NUT); published and unpublished articles; education pamphlets; and newspaper clippings of articles and editorials related to her dispute with the Board of Education and on general educational topics.