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The collection includes Schiller's notebooks, his working notes, scripts of his lectures, articles and essays, correspondence concerning engagements and with colleagues and students, material relating to his involvement with courses for teachers, personalia, printed material and photographs. Schiller's notebooks mainly contain working notes and the text for his lectures which provide evidence of his educational ideas, for instance, on the teaching of numbers, the importance of freedom and creativity through art, craft and movement activities, on reading, writing and conversation.
Also included are the notes and papers of Schiller's wife, Mrs Lyndall Schiller, including diaries of their daughters' childhood development. These records of Lyndall were deposited along with those of her husband and as much of them relate to matters that were of interest to both of them they have been retained within the collection of her husband's papers.
In addition the collection contains papers of two of Schiller's students who attended the 'Course on the Education of Children in the Junior School' organised by Christian Schiller at the University of London Institute of Education, 1959s. These include some wooden mathematical teaching apparatus.

Papers regarding Cynthia Reynolds career as an advisory teacher for the Inner London Education Authority (ILEA) including, writings by Cynthia Reynolds, including reports for the ILEA and published writings, 1970-1983; papers regarding home economics curriculum development in secondary schools, 1945, 1968-1983, including sample syllabuses and exam papers from across the UK and overseas, development of in-service courses for teachers, ILEA publications and general files on curriculum development with reference to home economics; papers regarding the development for parenting courses in secondary schools, 1963-1985, including development within the ILEA, developments outside London and writings about parenting courses; Health and Nutrition education publications from the ILEA and other local education authorities, 1972-1985; ILEA lower school projects in home economics, 1979-1983; papers regarding home economics in further education, 1972-1985, including Reynolds MA dissertation; and general publications on home economics education.

Papers of Susan Sutherland Isaacs, 1928-1979, including personalia; some correspondence relating to students at the Institute of Education, University of London, 1933-1939; press cuttings relating to her writings as 'Ursula Wise' from the journals Nursery World and Home and School, 1929-1940; a few published papers, articles and drafts, notably of An introduction to psychology (Methuen, London, 1928).

Papers of Nathan Isaacs, 1913-1966, including lectures, unpublished writings and notes, publications and correspondence concerning his psychological and philosophical work.

Papers of Dorothy Ellen Marion Gardner including annual reports of the Child Development Department at the Institute of Education, University of London, 1933-1958, and notes on its establishment and functioning; newsletters of the Child Development Society, 1950-1992; pamphlets relating to child development issues, 1945-1960; correspondence and papers relating to reading skills, [1962-1963]; correspondence and papers relating to Dorothy Gardner's memorial meeting and fund, 1972-1976.

Papers relating to the work of Amelia Fysh (nee Bullen), mainly at Beech Green Nursery School, Aylesbury, Bucks. Much of the material relates to her work on the relation of children's drawings to their development and includes originals and photocopies of the children's drawings, photographs of the children playing and working at the nursery school, and Amelia's research notes, papers and correspondence regarding her efforts to get the work published. The collection includes a copy of her publication 'Discovering Development with the 3-5s: a longitudinal study, 1964-1973', published c1997.

There are a number of personal files relating to Amelia's own education, her career in education provision, and her research into child development in other countries. These latter papers appear to have been created on an ad hoc basis during her travels abroad. There are also a number of publications regarding child development, pre-school education and education for children with learning and physical disabilities.

Records of the Child Development Society, 1942-2004, comprising administrative material relating the management of the Society, including the constitution of the Society, 1942-1994; minutes and circulated papers of meetings of the Executive Committee and Annual General Meetings, 1988-2003; correspondence of Annabel Lewis, Chair of the Society, from members of the Society and external bodies, 1996-2004; membership lists, 1993-[2000]; material relating to events held by the Society including programmes, literature, publicity, and correspondence, 1985-2000; promotional literature including the Society's newsletter and leaflets advertising the Society, 1972-2004; and miscellaneous material, including a note book, press cuttings and articles, 1992-[2002].