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The collection comprises manuscript notebooks, printed pamphlets, correspondence, a minute book, and photographic and other catalogues, 1768-1970. These notably include notebooks containing descriptions and viewing data relating to astronomical observations carried out at Kew Observatory, Richmond, Surrey, on behalf of King George III, with a printed pamphlet by Nevil Maskelyne, Astronomer Royal, entitled Observations of the transit of Venus over the Sun, 1768-1769; manuscript notebook containing measurements recorded during a test of the accuracy of the H5 chronometer designed by John Harrison, 1772; manuscript notebooks recording daily temperature, barometric, hygrometric and rainfall readings taken at Kew Observatory, Richmond, Surrey, 1773-1840; a printed pamphlet by George Atwood, Fellow of the Royal Society, entitled A Supplement to 'A treatise on the construction and properties of arches' (London, 1804), with manuscript dedication to King George III and related correspondence, 1804-1805; a folio signature book of visits by dignitaries to the George III Museum, 1843-1929; manuscript diary describing the work of the George III Museum including the upkeep of equipment and use of exhibits in experiments, 1850-1880; manuscript minutes of the George III Museum Committee charged with managing the collection, 1880-1885; catalogues relating to the collection, [1841-1970]; correspondence by George Calver, astronomer, relating to telescope design, 1897; series of copper plates and labels advertising the George III Museum, [1841-1926].

Chelsea College Library records, 1895-1987, comprise papers collected by the College Library or describing the work of the Library on the Chelsea campus following the merger with King's College in 1985, notably correspondence with the College Secretary and departments, 1974-1980; papers relating to Library computerisation, 1979-1987; staffing and salary matters, 1978-1985; University Grants Committee papers on libraries, 1974-1982; History and Philosophy of Science Library correspondence and bibliography, 1964-1987; Chelsea Campus Libraries Users Committee notes, 1985-1987; finance, 1975-1977; concerning the College History Collection, 1965-1974; notes relating to building and planning at the King's Road site, 1971-1987; University of London merger and other papers, 1978-1983; reports on medical education in London, 1980; concerning Library private papers, 1949-1970; Library Annual Reports, 1963-1987 (1992/CAL, CAL/1986); correspondence concerning Library donors and Zoology reprints, 1967-1985 (Ref: 1986/CAL); accessions registers, 1921-1975 (Ref: CAL/RG); lists of current periodicals, 1960-1974 (Ref: CAL/RGJ); payments books for stock, equipment and expenses, 1960-1973 (Ref: CAL/CB); Library staff personnel files for leavers between 1970-1976 (Ref: CAL/FP); material concerning the history of the College accumulated by the Library, including charters, official reports, with some press cuttings, 1914-1981 (Ref: CAL/H).

Records, c1869-1979, of the Strand School and its predecessors, comprising Headmaster's general and policy files, 1875-1977 (Ref: KSS/GPF); minutes of the Strand School, 1913-1938, and minutes relating to staff, 1957-1978, Houses of the school, 1942-1969, school societies, 1936-1957, parents' open evenings, 1956-1969, and conference of Headmasters and mistresses of London County Council (LCC) secondary schools, 1925-1952 (Ref: KSS/M); ledgers of pupils' accounts with the school, 1868-1908 (Ref: KSS/L); printed school accounts, 1910-1913 (Ref: KSS/ACC); registers containing staff details, 1893-1970, pupils' details, 1900-1925, 1931-1936, 1946-1979, and House records, 1933-1959 (Ref: KSS/R); Headmaster's albums of commended essays and artwork, 1912-1929 (Ref: KSS/ALB); record books of the Nature Society, 1909-1939, and sports record book, 1950-1956 (Ref: KSS/RB); programmes for school events, 1905-1912, 1950-1973, and school calendars, 1969-1977 (Ref: KSS/PRG); school magazines, 1905-1977 (Ref: KSS/PM); school prospectuses, 1915, 1938 (Ref: KSS/SYL); catalogues of books in Strand School and King's College use, c1869-c1894 (Ref: KSS/CA); bound addresses of thanks from staff and students to William Braginton, 1909-1910 (Ref: KSS/SP); private papers of Lt H Alnwick, comprising exercise books of plays written by him, 1924 (Ref: KSS/PP); ephemera including various invitation cards to school events, 1912, 1957-1968, a scheme for amalgamation of schools, 1906, regulations regarding management of the school, 1909, and the Strand School song and school rules, both undated (Ref: KSS/EPH); photographs, c1900-c1970 and undated, including school classes, staff, sports, portrait of William Braginton and the front of the Strand School, Brixton (Ref: KSS/PH); LCC's London School Plan and associated maps, 1947 (Ref: KSS/PBN); Keith Thomas White, 'History of Strand School, 1875-1913', written for MA in Science Education, Chelsea College, University of London, 1984 (Ref: KSS/TH).

Collection comprises correspondence with Philip Hammersley Leathes, manuscript papers, diaries, devotionals, dictionaries and pedigree rolls, title deeds and indentures, printed books and pamphlets, catalogues and the manuscripts of the architect, John Carter, [1350-1863]. Notably including correspondence from George Nayler of the College of Arms and Nicholas Carlisle, Secretary of the Society of Antiquaries, relating to publications of the Society, discoveries of antique brass plate, and the exchange of manuscripts between antiquaries, [1790-1838]; loose manuscript papers collected by Leathes, describing ornamentation in early printed devotionals, a fictional narrative entitled 'The amorous Jill: A tale', narrative of the Lisbon earthquake of 1755, notes relating to the observation of comets, including the comet of 1811, copies of charters of the reigns of Edward IV and Henry VII, papers relating to the Portland Vase, British Museum, fragments describing inscription on newly discovered brass plate, 1747-1829; pedigree rolls tracing the lineage of the English Crown, [1450, 1762]; manuscript volumes including collection of biblical extracts, liturgical handbook, autograph book with colour illustrations, antiquarian ephemera such as funeral memorials, armorials and the creation of nobles, volume by Francis Harrison entitled, 'The elements of navigation' with colour charts, tables and illustrations, dictionaries of Celtic and Saxon words, notes on the teaching of mathematics, commonplace book drawing on ancient and modern authors, manuscript diary including progress of architectural tour of Europe; title deeds and indentures for families in Nottingham, Southampton, London and Hungerford, residency certificates in Buckinghamshire and Northamptonshire, 1650-1751; printed books and pamphlets on the subjects of antiquarianism, genealogy and architecture, 1778-1853; manuscripts of John Carter, architect, acquired at his death in 1817 by his executor, Leathes, notably including autobiographical notebooks by Carter describing architectural subjects and tours, commonplace book, correspondence with Leathes, loose notes on linguistics and the ships of the Russia Company, obituaries of Carter and sale catalogue from his estate, 1700-1818; manuscript catalogues and display captions relating to the Leathes' papers, King's College London, 1819, 1837.

Experimental notes, working papers, correspondence and lecture summaries compiled by Charles Wheatstone, 1836-1875, and photographs collected by him in that period. Notably including papers relating to the development and testing of the telegraph, [1836-1960]; descriptions of experiments and test results concerning the measurement of electromotive forces and electrical potential, [1840-1875]; experimental observations on the nature of magnetism, electricity and thermodynamics, including electromagnet design, batteries and dynamos, [1834-1855]; working papers relating to optics including experiments into refraction, colouration of compounds and polarisation, [1850-1875]; drafts of lectures on sound and musical instruments prepared by Wheatstone, [1832-1837]; material relating to the management of the Wheatstone collection of scientific instruments and library, 1890-1992; biographical material relating to the life of Wheatstone, the invention of the telegraph and Wheatstone's musical instrument manufacturing business, with unrelated newspapers, 1757-1975; stereoscopic photographs and glass negatives taken by Roger Fenton, Samuel Buckle, Jules Duboscq and others, featuring landscapes, still lifes, panoramic scenes of cities including Paris and Moscow and the interior and exterior of the Crystal Palace, Hyde Park, Sydenham, 1851, and especially the Exposition Universelle, Paris, 1855, [1850-1901]; artefacts on loan from Department of Physics, King's College London, including telegraph apparatus, a nail fiddle and other prototype musical instruments, [1834-1875]; exhibition of scientific and musical instruments, [1834-1875].