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The Brain archive comprises his personal and professional papers together with sampled case notes from his private practice, 1865-1977. As well as medical papers, there is a significant amount of material relating to Brain's philosophical and literary interests, and some papers of Brain's family and of his wife Stella (nee Langdon-Down).

Sir James Paget's index to references for medical biographies, intended for the Biographical Dictionary of the Society for the Diffusion of Useful Knowledge (1842-44), c.1844.