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Sir Henry Head's papers, 1891-1909, consist of his casebooks of patients with Herpes Zoster, with sketches and photographs, chiefly from Head's work at the London Hospital, 1891-1909, and his casebooks of patients with various diseases, with sketches and charts, from his work at the City of London Hospital for Diseases of the Heart and Lungs, Victoria Park, 1894.

The Brain archive comprises his personal and professional papers together with sampled case notes from his private practice, 1865-1977. As well as medical papers, there is a significant amount of material relating to Brain's philosophical and literary interests, and some papers of Brain's family and of his wife Stella (nee Langdon-Down).