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Material relating to Bedford College Library, 1849-85, notably Minutes of the Library Committee, 1886-1983; Library working files, 1918-1985, on subjects including war arrangements, grant, University libraries, estimates and expenditure, staff and salaries and departmental matters; correspondence between the Librarian and the Secretary of the Council, 1889-1950; Library correspondence relating to alterations and repairs, 1932-1954; Library lists and registers, 1849-1985, including a Visitors' Book, 1953-1985, and Withdrawals Registers, 1917-1922 and 1954-1974; papers relating to insect problems in the Library, 1951; Doris Bains's statistics book and Library Staff Book; miscellaneous literary works, [1940-1959]; University Grants Committee (UGC) liaison reports, 1964; papers relating to the reclassification of the Library stock, 1969-1970; Library Accessions Register, 1897-1971; Pamphlet Accessions Register, 1921-1971; Donations Register, 1963-1970; plans by Maxwell Ayrton relating to the Tate Library extension, 1932-1950; plans by Easton and Robertson relating to the Tate and Herringham Library extension, 1961-1963.

Reports and publications of the Library, 1892-1984, including Annual Reports, 1965-1984; Stock Books, 1892-1976; Registers of Gifts, 1889-1967; Registers of books requested, 1893-1933. Papers and plans relating to the Library, 1944-1970, notably reports, plans and tables relating to the reorganisation of the Library, 1964-1965; report, provisional estimate, memoranda and plans relating to a proposed extension to the Library, 1970. Material relating to Library committees, 1949, 1965-1967, including the Archives Sub-Committee and the Library Representatives Committee. Personnel files relating to former Library Staff, 1952-1974. Library accounts books, 1948-1971. Material relating to Library accessions and donations.

Staff files, 1900-1985, containing information relating to employment issues such as applications, appointment letters, correspondence, and information on salary and superannuation; correspondence with the University of London, 1908-1961; material relating to the appointment of staff, including the Principal, 1929 and 1971, research staff, 1921-1953, Library Assistants, 1912-1948, administrative Assistants, 1927-1946, and Laboratory Assistants, 1912-1939; papers relating to Staff appointments and conditions, 1906-1918 and 1940; papers concerning the restructuring of pay and duties of Laboratory Technicians, 1973; papers regarding the employment of postgraduates in science research, 1962-1964; material on war, disablement and sickness benefits, 1919-1955; papers on appointments to Chairs and Readerships, 1919-1960; papers of the Sub-Committee on Secretarial and Clerical Staff, 1968-1972; Minutes, papers and reports of the Department Staffing Committees, 1946-1976.