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Original manuscripts of letters to the Royal Society, which are largely scientific. These papers form the raw material from which the Letter Books were compiled. There are many letters of importance, 1613; 1642; 1651-1740.

Correspondence, diaries and other papers of Sir Alfred Charles Glyn Egerton, including some personal papers but largely relating to The Royal Society and particularly to wartime activities and post-war research needs in Britain. The diaries form an almost complete record of Egerton's career during the period 1943-1959. Earlier diaries date back to 1917 and the period 1929-1930, but for the most part they relate to the period 1938-1941.

Papers relating to the International Association of Academies including Generalplan zur Grundung einer internationalen Association der Akademien, 1899; Statuten der internationalen Assoziation der Akademien, 9-10 October 1899; Letter from J Larmor, Secretary of the Royal Society, to the President of the Council of the International Association of Academies, Imperial Academy of Sciences, Vienna 21 December 1905; Letter from Chevalier Edm. Marchal, Secretaire perpetuel de l'Academie Royale des Sciences, des Lettres et des Beaux-Arts de Belgique, 16 May 1905; Letter from Robert Harrison, Assistant Secretary of the Royal Society to The President, Kaiserliche Akademie der Wissenschaften, Vienna, 14 February 1906; Letter from J Gollancz, Secretary of the British Academy to Professor Victor von Lang, 26 February 1906; Letter from Robert Harrison to Professor Arthur Schuster FRS, 16 March 1906; Minutes of first sitting of General Assembly of the International Association of Academies, 29 May 1906; Minutes of the Committee meeting held on, 1 June 1906.

Working papers and correspondence of Sir Francis (Franz) Eugene Simon. Scientific notebooks in the collection date from 1919-1934, largely the period of Simon's researches on low temperature physics at the Physikalisch-Chemisches Institut of Berlin University, and subsequently at Breslau. Other notes and manuscripts for lectures and articles are post 1930, while a large group of correspondence files are from the years 1922-1956, providing a full account of Simon's dealings with many fellow scientists and scientific organisations. Individual letter files concern V.M. Goldsmidt, Max Born, Gwyn Owain Jones and Nevill Mott among many other notable figures. Details of Simon's involvement in atomic energy development are to be found in papers on uranium isotope separation (MAUD Committee notes) and UK Atomic Energy Authority correspondence. Simon's professional appointments as head of the Clarendon Laboratory and as science correspondent to the Financial Times are represented by substantial groups of letters. There are twelve notebooks with some associated papers; the series also includes files of lectures, articles, cuttings and souvenirs, including photographs, with files of correspondence. Two later additions to the collection consist of correspondence and files highlighting Simon's contacts with industrial firms, universities and international organisations.

A small collection of papers of Sir Arthur George Tansley, mainly related to the formation of organisations, in the period 1918-1921, that aimed to promote pure and applied scientific research. The bulk of the collection consists of papers relating to Tansley's involvement in the Scientific Research Association. The Scientific Research Association's papers include rules, promotional leaflets and circulars, financial material and a relatively large amount of correspondence. A smaller amount of material survives for the National Union of Scientific Workers including rule booklets, membership lists, reports from meetings, agenda and promotional leaflets and circulars. Only a few items are preserved in this collection for the Federation of Technical and Scientific Associations and the Cambridge Research Group. The published articles and reports at AT/5 mainly concern issues related to the funding, support and the general state of scientific research. As a whole the collection reveals many problems faced by those who wished to organise research work after the first world war, such as the problem of rival organisations created to promote research whose aims overlapped, and disagreements over how and whether research could be organised. For example a letter from the Royal Society to the Scientific Research Association commented that 'lines of development' were 'discovered not by councils or committees but by the instinct of individuals, and the less this is trammelled by organization the better' (AT/2/6/1/42). The article 'Research and Organisation' at AT/2/3/15 was written in an attempt to answer such criticisms by arguing that research could be organised. Other issues also surface in the correspondence of the Scientific Research Association. For example one letter opposed support for any scheme founded on government funding as 'government endowment will, in the long run, corrupt Science...' (AT/2/6/2/17). There were also disagreements as to whether emphasis should be laid upon 'the promotion of scientific research' or 'the economic interest' of research workers which seems to have contributed to a division between the National Union of Scientific Workers and the Scientific Research Association (AT/2/4/3).