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Scientific and other papers sent to the Royal Society, presented at meetings of Fellows, or commissioned by the Society. They form a complementary series to the Early Letters, both of which were superseded by the Letters and Papers. Many of these items, referred to as the 'Guard Books', are duplicated in the Register Book of the Society. The classification is a simplified form of the 'Philosophical Transactions' abridgment by John Lowthorp. This arrangement was completed in 1741 by Thomas Birch. The majority of the papers in these volumes are manuscript, but a few printed documents occur throughout the series. Some of the papers are earlier in date than the grant on 15 July 1662 of the First Charter to the Society. The Committee of Trades seems to have been associated with the earlier meetings of those philosophers who subsequently became Fellows, and produced a number of practical papers, some of which were written in 1639 and which are mostly found in Volume 3(i). There are still earlier documents, mostly in Volume 25, which may have been included in the gift, in 1667, of the Arundel Library.

Letters from Sir Robert Moray to his friend Alexander Bruce, Earl of Kincardine, also known as 'The Kincardine Papers'. Bruce was sick of the ague in Bremen for part of this time, and the letters were written to alleviate the tedium of of Bruce's illness, hence ranging over topics which might not otherwise have been the subjects of correspondence. They include accounts of chemical experiments in his laboratory, his interest in magnetism, medicine in all its aspects, horticulture, fuel, whale fishing, its risks and profits, coal mining, water wheels and tide mills, stone quarrying and the various qualities of different stones, the pumping works needed for undersea coal mines at Bruce's home at Culross in Fifeshire, even to the trees whose wood was best for pipelines, and the diameter of the bore best suited to the purpose. Familiarity is shown with mathematical and surveying instruments, with music, and all sorts of mechanical devices and especially clocks and watches, more particularly the taking out of a patent in respect of a clock for use at sea for finding longitude. Bruce is advised on the choice of books over a wide range of subjects. Moray includes anecdotes to amuse his ailing correspondent; he describes his quiet life and is enthusiastic about many of his chemical experiments. Notable at the end of the letters Moray added what he described as his Masonic signature - a pentagram which also occurs in his crest.