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The papers consist of notes and notebooks of William Bayliss' experiments. There is also correspondence, press cuttings and photographs, a great part referring to the 'Brown Dog Affair' of 1903 and to other disputes between anti-vivisectionists and University College London.

Letterbooks of Sir Isaac Lyon Goldsmid, 1805-1856 and undated but dating largely from the period 1828-1835, mainly comprising letters to Goldsmid concerning his interests and activities in Jewish emancipation, social and educational reform, including the foundation of the University of London. The writers (c350 in total) include Henry Addington, 1st Viscount Sidmouth, 1830, 1833; Peter Bedford, 1832; Henry Peter Brougham, Baron Brougham and Vaux, 1828-1839 and undated; Sir Francis Burdett, Baronet, 1830, 1833; Benjamin Disraeli, 1st Earl of Beaconsfield, 1835 and undated; Michael Faraday, 1831; Henry Richard Vassall Fox, 3rd Baron Holland, 1828-1840 and undated; Elizabeth Fry, 1829, 1833 and undated; Sir Robert Grant, 1830-1834 and undated; Charles Grey, 2nd Earl Grey, 1832-1834; William Lamb, 2nd Viscount Melbourne, 1835; Thomas Babington Macaulay, Baron Macaulay, undated; Thomas Robert Malthus, 1827; Harriet Martineau, 1834 and undated; Daniel O'Connell, 1829; Robert Owen, 1830 and undated; David Ricardo, 1823; Henry John Temple, 3rd Viscount Palmerston, 1834-1841; Arthur Wellesley, Duke of Wellington, 1828, 1833; and many other public figures including politicians, aristocrats, members of the royal family, reformers, churchmen, and prominent Jewish figures. There are a few letters from Goldsmid, 1828-1856 and undated, and other documents, including one concerning places of worship in Old and New Lanark, 1823; London University share certificate, 1826; and a copy petition to (Sir) Robert Grant on behalf of the Jewish Disabilities Bill, 1833.

Letters from Grote to Sir William Smith, lexicographer, concerning Smith's work and Grote's History of Greece, plus other subjects. Also included is a printed notice by Joseph Mazzini dated 8 November 1852, appealing for money, and a duplicated circular letter to Grote relating to 'The Hungarian Fund', signed by Lajos Kossuth, with a note from Grote, 1853.

Papers of and relating to the Horsley family, comprising papers of Sir Victor Horsley; papers of Eldred, Lady Horsley; papers of Siward Horsley and of Oswald Horsley; papers of Pamela, Lady Robinson, including items relating to the Babies Club in Chelsea; papers of Stephen Paget, author of Victor Horsley's biography; photographs and postcards. Victor Horsley's papers include large sections on his medical career, his service in the army during the Great War, and his political and social interests, including his involvement in the temperance movement and the Medical Defence Union, support for the suffragettes and for Home Rule for Ireland, and his role in the reform of the bodies representing the medical profession: the General Medical Council, the British Medical Association, and the Royal College of Surgeons. His personal papers reflect his interest in archaeology and genealogy.

Photocopies of correspondence with the Hungarian politician Ferencz Aurelius Pulszky.