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Papers of Dr. Letitia Fairfield, reflecting her interests in social hygiene, in mental health, in medico-legal matters and criminology, mother and child health and welfare, and as a Roman Catholic convert, as well as her broader political and feminist convictions. There is also some biographical material.

Sargant was an outspoken supporter and practitioner of what he termed the 'practical rather than philosophical approaches' to the treatment of mental illness, pioneering and publicising various physical treatments and vociferously opposing the use of psychoanalytic techniques. The majority of the collection consists of his writings, both published and unpublished, supplemented by a small quantity of correspondence and other material. In addition, the collection contains clinical records for about 500 cases from Sutton Emergency Hospital in the 1940s. As well as covering clinical subjects (in Sections D, E, and F) and Sargant's views on the practice of psychiatry in general (Section B), the collection also contains material relating to his interest in the related issues of religious conversion and brainwashing (Section G).