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The collection chiefly comprises correspondence by Florence Nightingale, either in original or in copy form. The date-span covers the whole of her life and the subjects range from her attempts to become a nurse, service in the Crimea and subsequent work reforming the training and practice of nursing, through her other concerns such as Indian sanitation, cottage hospitals and the use of medical statistics, to personal and family matters. Well-represented correspondents include her family (particularly her sister Parthenope and brother-in-law Sir Harry Verney), Sir William Aitken (1825-1892), Professor of Pathology at the Army Medical School; George Hanby De'ath (c.1862-1901), Medical Officer of Health for Buckingham; William Farr (1807-1883), statistician; Miss Louisa Gordon, Matron at St Thomas' Hospital; Miss Amy Hughes, Superintendent of the Nurses' Co-operation; Sir John Henry Lefroy (1817-1890); Charles C. Plowden of the Sanitary Department of the India Office; and Mary Clarke Mohl (1793-1883). In addition, there is twentieth century material relating to Nightingale's legacy such as photographs of her grave (at MS.9101) and administrative papers relating to the compilation of A calendar of the letters of Florence Nightingale (Oxford, 1977) by Sue Goldie (MSS.9106-9109).

Correspondence and papers of the statesman Henry Dundas both general and in his capacity as Commissioner (later President) of the Board of Control, 1783-1811.

Notes by John Dixon on medical matters and on things of personal interest to him such as astrology and photography spanning his entire career, 1848-1903. MS.5191 comprises more formal material, namely certificates and indentures.