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The collection covers both Pettigrew's medical and antiquarian activities, which are intermingled in the material's arrangement. The medical items include correspondence with many medical figures, medical jurisprudence (an Anniversary Oration delivered to the Medical Society of London), corpulence, hydrophobia, medical observations by army officers in India, and an autobiographical memoir of the philanthropist and prison-reformer James Neild (1744-1814), transcribed by Pettigrew and incorporated into his life of John Coakley Lettsom M.D. The antiquarian items include material on Kett's Rebellion, Hindu deities, the library of the Duke of Sussex and correspondence with the Italian antiquary Giovanni Spano (1803-1878) and Gaetano Cara, as part of Pettigrew's role as Vice-President of the British Archaeological Society. Types of material held include notebooks, loose papers, correspondence and diplomas.

Papers of Jean Nicholas Marjolin and his son René Marjolin, 1849-1894, including notes of Jean Nicolas Marjolin's lectures, by a medical student; letters from René Marjolin to his friend Edmond Dascols relating mainly to personal affairs, and the health of the Dascols family (with advice on cholera and other maladies) and letters from Paris at the time of the siege and the Commune, 1870-1871, when René Marjolin was active in treating the wounded prior to his arrest as a Bonapartist agent.

Manuscript translation into English, by an unknown hand, of Petrus Martyr Anglerius, Opus epistolarum ... Cui accesserunt epistolæ Ferdinandi de Pulgar, Latinæ pariter atque Hispanicæ (in Latinum idioma conuersæ a J. Magon), cum tractatu Hispanico de viris Castellæ illustribus, edited by C. Patin, (Elsevir, Amsterdam, 1670) 'The Work of the Letters of Peter Martyr of Angleria, a Milanese...to which are added the letters of Fernandez de Pulgar....'.